Weakly-Correlated Nature of Ferromagnetism in Nonsymmorphic CrO_{2} Revealed by Bulk-Sensitive Soft-X-Ray ARPES

Weakly-Correlated Nature of Ferromagnetism in Nonsymmorphic CrO_{2} Revealed by Bulk-Sensitive Soft-X-Ray ARPES

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Chromium dioxide CrO_{2} belongs to a class of materials called ferromagnetic half-metals, whose peculiar aspect is that they act as a metal in one spin orientation and as a semiconductor or insulator in the opposite one.Despite numerous emtek freestone finger pull experimental and theoretical studies motivated by technologically important applications of this material in spintronics, its fundamental properties such as momentum-resolved electron dispersions and the Fermi surface have so far remained experimentally inaccessible because of metastability of its surface, which instantly reduces to amorphous Cr_{2}O_{3}.In this work, we demonstrate that direct access to the native electronic structure of CrO_{2} can be achieved with soft-x-ray angle-resolved photoemission spectroscopy whose large probing depth penetrates through the Cr_{2}O_{3} layer.For the first time, the electronic dispersions and Fermi surface of CrO_{2} are measured, which are fundamental prerequisites to solve the long debate rohrventilator industrie on the nature of electronic correlations in this material.Since density functional theory augmented by a relatively weak local Coulomb repulsion gives an exhaustive description of our spectroscopic data, we rule out strong-coupling theories of CrO_{2}.

Crucial for the correct interpretation of our experimental data in terms of the valence-band dispersions is the understanding of a nontrivial spectral response of CrO_{2} caused by interference effects in the photoemission process originating from the nonsymmorphic space group of the rutile crystal structure of CrO_{2}.